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Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)

Polyhydroxyalkanoates (PHAs) are microbial polyesters produced by many types of bacteria as an intracellular energy reserve material under substrate limiting conditions and in the presence of excessive carbon sources.¹ Poly((R)-3-hydroxybutyrate) (PHB), the most commonly used microbial polyester, wa...

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Главные авторы: Rajaratanam, Dhurga Devi, Ariffin, Hidayah, Hassan, Mohd Ali, Nishida, Haruo
Формат: Статья
Язык:English
Опубликовано: Nature Publishing Group 2016
Online-ссылка:http://psasir.upm.edu.my/id/eprint/55245/1/Changes%20in%20diad%20sequence%20distribution%20by%20preferential%20chain%20scission%20during%20the%20thermal%20.pdf
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spelling oai:psasir.upm.edu.my:55245 http://psasir.upm.edu.my/id/eprint/55245/ Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) Rajaratanam, Dhurga Devi Ariffin, Hidayah Hassan, Mohd Ali Nishida, Haruo Polyhydroxyalkanoates (PHAs) are microbial polyesters produced by many types of bacteria as an intracellular energy reserve material under substrate limiting conditions and in the presence of excessive carbon sources.¹ Poly((R)-3-hydroxybutyrate) (PHB), the most commonly used microbial polyester, was the first member of the PHA family to be discovered, and more than 150 other monomer units have been reported to date.2, 3 Poly((R)-3-hydroxybutyrate-co-(R)-3-hydroxyhexanoate) (PHBHHx) is a copolymer in the PHA family that consists of randomly distributed (R)-3-hydroxybutyrate (HB) and (R)-3-hydroxyhexanoate (HHx) units.⁴ This type of copolymer exhibits improved mechanical properties and processability compared with those of PHB and poly((R)-3-hydroxyvalerate) (PHBV).⁵ PHBHHx copolymers are currently produced on a large scale and have proven to be biocompatible in clinical studies using mouse fibroblasts cells, and rabbit articular cartilage-derived chondrocytes.⁶ PHBHHx is a highly favorable copolymer of the PHB family due to its biodegradability, flexible mechanical properties and good melt processability. Nature Publishing Group 2016 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/55245/1/Changes%20in%20diad%20sequence%20distribution%20by%20preferential%20chain%20scission%20during%20the%20thermal%20.pdf Rajaratanam, Dhurga Devi and Ariffin, Hidayah and Hassan, Mohd Ali and Nishida, Haruo (2016) Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate). Polymer Journal, 2016 (NA). pp. 1-4. ISSN 0032-3896; ESSN: 1349-0540 10.1038/pj.2016.28
institution UPM IR
collection UPM IR
language English
description Polyhydroxyalkanoates (PHAs) are microbial polyesters produced by many types of bacteria as an intracellular energy reserve material under substrate limiting conditions and in the presence of excessive carbon sources.¹ Poly((R)-3-hydroxybutyrate) (PHB), the most commonly used microbial polyester, was the first member of the PHA family to be discovered, and more than 150 other monomer units have been reported to date.2, 3 Poly((R)-3-hydroxybutyrate-co-(R)-3-hydroxyhexanoate) (PHBHHx) is a copolymer in the PHA family that consists of randomly distributed (R)-3-hydroxybutyrate (HB) and (R)-3-hydroxyhexanoate (HHx) units.⁴ This type of copolymer exhibits improved mechanical properties and processability compared with those of PHB and poly((R)-3-hydroxyvalerate) (PHBV).⁵ PHBHHx copolymers are currently produced on a large scale and have proven to be biocompatible in clinical studies using mouse fibroblasts cells, and rabbit articular cartilage-derived chondrocytes.⁶ PHBHHx is a highly favorable copolymer of the PHB family due to its biodegradability, flexible mechanical properties and good melt processability.
format Article
author Rajaratanam, Dhurga Devi
Ariffin, Hidayah
Hassan, Mohd Ali
Nishida, Haruo
spellingShingle Rajaratanam, Dhurga Devi
Ariffin, Hidayah
Hassan, Mohd Ali
Nishida, Haruo
Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
author_facet Rajaratanam, Dhurga Devi
Ariffin, Hidayah
Hassan, Mohd Ali
Nishida, Haruo
author_sort Rajaratanam, Dhurga Devi
title Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
title_short Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
title_full Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
title_fullStr Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
title_full_unstemmed Changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
title_sort changes in diad sequence distribution by preferential chain scission during the thermal hydrolysis of poly(3-hydroxybutyrate-co-3-hydroxyhexanoate)
publisher Nature Publishing Group
publishDate 2016
url http://psasir.upm.edu.my/id/eprint/55245/1/Changes%20in%20diad%20sequence%20distribution%20by%20preferential%20chain%20scission%20during%20the%20thermal%20.pdf
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score 13.4562235

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